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Green hydrogen recovery from natural gas grids by adsorption process

2023Conference object Open access
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dc.contributor.authorZafanelli, Lucas F.A.S.
dc.contributor.authorAly, Ezzeldin
dc.contributor.authorHenrique, Adriano
dc.contributor.authorRodrigues, Alírio
dc.contributor.authorSilva, José A.C.
dc.date.accessioned2025-01-20T12:25:26Z
dc.date.available2025-01-20T12:25:26Z
dc.date.issued2023
dc.description.abstractIn this work, the binder-free zeolite 13X was tested to purify green hydrogen injected into natural gas grids. Green hydrogen can be a key factor in meeting global energy demand while contributing to climate goals. In this way, breakthrough curve experiments were performed to assess the equilibrium and kinetic adsorption for H2 and CH4 in binder- free zeolite 13X. This work covers the lack of adsorption data and multicomponent breakthrough curves of H2/CH4 at low temperatures (until 195 K) which were not available in the literature. The equilibrium data were modeled by using the dual-site Langmuir isotherm model and the multicomponent breakthrough curves were simulated using a mathematical model implemented in MATLAB. Performance parameters based on equilibrium data were discussed. Overall, binder-free zeolite 13X has great potential to separate H2 from CH4 based on equilibrium (higher capacity for CH4 with fast diffusion of both gases).pt_PT
dc.description.sponsorshipThe authors are grateful to the Foundation for Science and Technology (FCT, Portugal) under project PTDC 2020 * 3599-PPCDTI * Engenharia dos Processos Químicos * project PTDC/EQU- EPQ/0467/2020. Also, through national funds FCT/MCTES (PIDDAC) to CIMO (UIDB/00690/2020 and UIDP/00690/2020), SusTEC (LA/P/0007/2021), ALiCE (LA/P/0045/2020), and LSRE-LCM (UIDB/50020/2020 and UIDP/50020/2020). Additionally, we thank national funding by FCT through the individual Ph.D. research grant SFRH/BD/7925/2020 of Lucas F. A. S. Zafanelli. Moreover, the authors are grateful to Kristin Gleichmann and Chemiewerk Bad Koestritz GmbH for kindly providing the binder-free beads of zeolite 13X studied in this work.pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.citationZafanelli, Lucas F.A.S.; Aly, Ezzeldin; Henrique, Adriano; Rodrigues, Alírio E.; Silva, José A.C. (2023). Green hydrogen recovery from natural gas grids by adsorption process. In Ana Maria Alves Queiroz da Silva; António Manuel Coelho Lino Peres; António Manuel Esteves Ribeiro; Maria Olga de Amorim e Sá Ferreira; Maria Filomena Filipe Barreiro; Paulo Miguel Pereira de Brito; Simão Pedro de Almeida Pinho (Eds.) 14th International Chemical and Biological Engineering Conference (CHEMPOR 2023): book of Abstracts. Bragança. ISBN 978-972-745-327-6pt_PT
dc.identifier.isbn978-972-745-327-6
dc.identifier.urihttp://hdl.handle.net/10198/31039
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherInstituto Politécnico de Bragançapt_PT
dc.relationGreen Hydrogen Separation from Natural Gas Grids by Adsorption Processes with MOFs
dc.relationMountain Research Center
dc.relationMountain Research Center
dc.relationALICE - Associate Laboratory in Chemical Engineering
dc.relationLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
dc.relationLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/pt_PT
dc.subjectGreen Hydrogenpt_PT
dc.subjectHydrogen Recoverypt_PT
dc.subjectHydrogen Purificationpt_PT
dc.subjectNatural Gas Gridspt_PT
dc.subjectZeolite 13Xpt_PT
dc.subjectProcess Simulationpt_PT
dc.titleGreen hydrogen recovery from natural gas grids by adsorption processpt_PT
dc.typeconference object
dspace.entity.typePublication
oaire.awardTitleGreen Hydrogen Separation from Natural Gas Grids by Adsorption Processes with MOFs
oaire.awardTitleMountain Research Center
oaire.awardTitleMountain Research Center
oaire.awardTitleALICE - Associate Laboratory in Chemical Engineering
oaire.awardTitleLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
oaire.awardTitleLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/Concurso para Financiamento de Projetos de Investigação Científica e Desenvolvimento Tecnológico em Todos os Domínios Científicos - 2020/PTDC%2FEQU-EPQ%2F0467%2F2020/PT
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oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F50020%2F2020/PT
oaire.citation.conferencePlaceBragançapt_PT
oaire.citation.endPage238pt_PT
oaire.citation.startPage237pt_PT
oaire.citation.title14th International Chemical and Biological Engineering Conference (CHEMPOR 2023): book of abstractspt_PT
oaire.fundingStreamConcurso para Financiamento de Projetos de Investigação Científica e Desenvolvimento Tecnológico em Todos os Domínios Científicos - 2020
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person.familyNameZafanelli
person.familyNameAly
person.familyNameHenrique
person.familyNameSilva
person.givenNameLucas F.A.S.
person.givenNameEzzeldin
person.givenNameAdriano
person.givenNameJosé A.C.
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person.identifier.orcid0000-0001-5187-2042
person.identifier.orcid0000-0003-4840-2597
person.identifier.orcid0000-0002-5227-9790
person.identifier.orcid0000-0003-1778-3833
person.identifier.scopus-author-id7403023684
project.funder.identifierhttp://doi.org/10.13039/501100001871
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project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
rcaap.rightsopenAccesspt_PT
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