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Performance and modeling of Ni(II) adsorption from low concentrated wastewater on carbon microspheres prepared from tangerine peels by FeCl3-assisted hydrothermal carbonization

2022Artigo científico Acesso aberto
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dc.contributor.authorDíaz de Tuesta, Jose Luis
dc.contributor.authorRoman, Fernanda
dc.contributor.authorMarques, Vitor da Costa
dc.contributor.authorSilva, Adriano S.
dc.contributor.authorSilva, Ana P. F.
dc.contributor.authorBosco, Tatiane
dc.contributor.authorShinibekova, Assem A.
dc.contributor.authorAknur, Sadenova
dc.contributor.authorKalmakhanova, Marzhan
dc.contributor.authorMassalimova, Bakytgul Kabykenovna
dc.contributor.authorArrobas, Margarida
dc.contributor.authorSilva, Adrián
dc.contributor.authorGomes, Helder
dc.date.accessioned2022-09-01T09:17:49Z
dc.date.available2022-09-01T09:17:49Z
dc.date.issued2022
dc.description.abstractThe presence of heavy metals in the environment as a consequence of human activity is an issue that has caught the attention of researchers to find wastewater treatment solutions, such as adsorption. In this work, hydrochars and activated carbon microspheres are prepared from tangerine peels as carbon precursor and FeCl3 as activating and structure-directing agent in the hydrothermal carbonization, allowing to obtain hydrochar microspheres ranging from 50 to 3615 nm. In addition, a pyrochar was prepared by pyrolysis of the same precursor. The activated carbon shows the highest surface area (SBET up to 287 m2 g–1), but the basicity of the pyrochar (1.83 mmol g-1, SBET = 104 m2 g–1) was determinant in the adsorption of Ni, being considered the carbon-based material with the highest uptake capacity of Ni. Isotherm and kinetic adsorption of Ni on the most representative activated carbon microsphere, pyrochar and hydrochar microsphere are assessed by 10 and 7 models, respectively.pt_PT
dc.description.sponsorshipThe authors are grateful to the FCT (Foundation for Science and Technology, Portugal) and FEDER (European Regional Development Fund) under Programme PT2020 for financial support to CIMO (UIDB/00690/2020). We would also like to thank the scientific collaboration under Base- UIDB/50020/2020 and Programmatic- UIDP/50020/2020 funding of LSRE-LCM, and LA/P/0045/2020 funding of ALiCE, funded by national funds through FCT and MCTES (Ministério da Ciência, Tecnologia e Ensino Superior, Portugal) by PIDDAC (Programa de Investimentos e Despesas de Desenvolvimento da Administraç˜ao Central, Portugal). Fernanda F. Roman and Adriano dos Santos Silva acknowledge the national funding by FCT and MIT (Massachusetts Institute of Technology, USA), and the ESF (European Social Fund) for individual research grants with reference numbers of SFRH/BD/143224/2019 and SFRH/BD/151346/2021, respectively.pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.citationDíaz de Tuesta, Jose Luis; Roman, Fernanda; Marques, Vitor C.; Silva, Adriano S.; Silva, Ana P.F.; Bosco, Tatiane C.; Shinibekova, Assem A.; Aknur, Sadenova; Kalmakhanova, Marzhan S.; Massalimova, Bakytgul K.; Arrobas, Margarida; Silva, Adrián; Gomes, Helder (2022). Performance and modeling of Ni(II) adsorption from low concentrated wastewater on carbon microspheres prepared from tangerine peels by FeCl3-assisted hydrothermal carbonization. Journal of Environmental Chemical Engineering. ISSN 2213-3437. 10:5, p. 1-15pt_PT
dc.identifier.doi10.1016/j.jece.2022.108143pt_PT
dc.identifier.issn2213-3437
dc.identifier.urihttp://hdl.handle.net/10198/25863
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherElsevier
dc.relationLA/P/0045/2020pt_PT
dc.relationMountain Research Center
dc.relationLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
dc.relationLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
dc.relationAdaptive Learning via Intuitive/Interactive, Collaborative and Emotional systems
dc.relationAmphiphilic carbon-based materials for one-pot desulfurization and denitrogenation of liquid fuels
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/pt_PT
dc.subjectHeavy metalpt_PT
dc.subjectCarbonaceous materialpt_PT
dc.subjectCitric peelspt_PT
dc.subjectWaste valorizationpt_PT
dc.subjectWastewater treatmentpt_PT
dc.subjectNonlinearpt_PT
dc.subjectError functionpt_PT
dc.subjectCircular economypt_PT
dc.titlePerformance and modeling of Ni(II) adsorption from low concentrated wastewater on carbon microspheres prepared from tangerine peels by FeCl3-assisted hydrothermal carbonizationpt_PT
dc.typejournal article
dspace.entity.typePublication
oaire.awardNumberUIDB/00690/2020
oaire.awardNumberUIDB/50020/2020
oaire.awardNumberUIDP/50020/2020
oaire.awardNumber257639
oaire.awardNumberSFRH/BD/143224/2019
oaire.awardNumberSFRH/BD/151346/2021
oaire.awardTitleMountain Research Center
oaire.awardTitleLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
oaire.awardTitleLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
oaire.awardTitleAdaptive Learning via Intuitive/Interactive, Collaborative and Emotional systems
oaire.awardTitleAmphiphilic carbon-based materials for one-pot desulfurization and denitrogenation of liquid fuels
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F00690%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F50020%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F50020%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/EC/FP7/257639/EU
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/POR_NORTE/SFRH%2FBD%2F143224%2F2019/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/POR_NORTE/SFRH%2FBD%2F151346%2F2021/PT
oaire.citation.issue5pt_PT
oaire.citation.startPage108143pt_PT
oaire.citation.titleJournal of Environmental Chemical Engineeringpt_PT
oaire.citation.volume10pt_PT
oaire.fundingStream6817 - DCRRNI ID
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oaire.fundingStream6817 - DCRRNI ID
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person.familyNameDíaz de Tuesta
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person.givenNameJose Luis
person.givenNameFernanda F.
person.givenNameAdriano S.
person.givenNameAna P. F.
person.givenNameMargarida
person.givenNameHelder T.
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person.identifier.ciencia-id991F-2DB8-3246
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person.identifier.ciencia-id6218-1E19-13EE
person.identifier.orcid0000-0003-2408-087X
person.identifier.orcid0000-0001-5360-5298
person.identifier.orcid0000-0002-6795-2335
person.identifier.orcid0000-0001-8979-8407
person.identifier.orcid0000-0002-4652-485X
person.identifier.orcid0000-0001-6898-2408
person.identifier.ridD-9785-2017
person.identifier.scopus-author-id55755821600
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project.funder.identifierhttp://doi.org/10.13039/501100001871
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project.funder.nameFundação para a Ciência e a Tecnologia
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project.funder.nameEuropean Commission
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