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Seasonal variation in exposure to particulate matter among children attending different levels of education: comparison of two dosimetry models

dc.contributor.authorCharres, Isabella
dc.contributor.authorCipoli, Yago Alonso
dc.contributor.authorFurst, Leonardo
dc.contributor.authorVicente, Estela D.
dc.contributor.authorCasotti Rienda, Ismael
dc.contributor.authorLazaridis, Mihalis
dc.contributor.authorFeliciano, Manuel
dc.contributor.authorAlves, Célia
dc.date.accessioned2024-07-31T14:32:47Z
dc.date.available2024-07-31T14:32:47Z
dc.date.issued2024
dc.description.abstractExposure to particulate matter (PM) has been associated with several adverse health outcomes. Studies indicate that children may be exposed to much higher concentrations of PM at school than in other environments. There exists very little data on the deposited dose of PM while children attend classes. This study was carried out in a school located near an industrial complex in Portugal and attended by children aged 3–12 years. Indoor PM10, PM2.5 and PM1 were measured over two seasons in classrooms representing different school year groups. Particle deposition fractions in the respiratory tract, as well as the deposited doses, were calculated using the Multiple-Path Particle Dosimetry (MPPD) and the Exposure Dose Model (ExDoM2). Both models were implemented assuming an 8-hour exposure scenario to represent the school day. In general, differences in PM concentrations were observed depending on room occupancy periods and season. The highest mean PM2.5 concentration was recorded in winter when the classroom was vacant (23.7 ± 20.5 μg m-3), while the highest mean PM10 level was observed in spring during school hours (61.7 ± 24.2 μg m-3). Regardless of the dosimetry model, the highest deposition of PM10 and PM2.5 was in the upper region, while the lowest was in the tracheobronchial (TB) region. The results indicate that deposited dose and deposition fraction in spring may be more harmful to pupils’ health than in winter. PM10 presented the highest doses, ranging from 54.2 to 128 μg and from 83.9 to 185 μg, according to MPPD and ExDoM2 estimates, respectively.pt_PT
dc.description.sponsorshipThe authors would especially like to thank the school principal, teachers, parents, and children who have willingly participated in this study. The help of Prof. Teresa Nunes, from the Department of Environment at the University of Aveiro, in interpreting the data is also appreciated. Special thanks to Owen Price from Applied Research Associates, Inc. for his support and expertise in answering questions related to MPPD. The authors acknowledge the financial support of the Portuguese Foundation for Science and Technology ( FCT ) to CESAM ( UIDP/50017/2020+UIDB/50017/2020+ LA/P/0094/2020 ), through national funds, and to the PhD fellows I. Charres (SFRH/BD/ 2022.12142 ), Y. Cipoli (SFRH/BD/04992/2021), L. Furst (SRFH/BD/08461/2020) and I. Rienda (SFRH/BD/144550/2019). FCT is also acknowledged for the research contract under Scientific Employment Stimulus to Estela D. Vicente (DOI:10.54499/2022.00399.CEECIND/CP1720/CT0012). This work was performed within the STEP project - Schools Tackling Estarreja's Air Pollution \u2013 funded by the LabEx-DRIIHM-OHM programme ( CNRS \u2013 INEE , France).pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.citationCharres, Isabella; Cipoli, Yago; Furst, Leonardo C.; Vicente, Estela D.; Casotti Rienda, Ismael; Lazaridis, Mihalis; Feliciano, Manuel; Alves, Célia (2024). Seasonal variation in exposure to particulate matter among children attending different levels of education: Comparison of two dosimetry models. Atmospheric Pollution Research. ISSN 1309-1042. 15:9, p. 1-12pt_PT
dc.identifier.doi10.1016/j.apr.2024.102229pt_PT
dc.identifier.issn1309-1042
dc.identifier.urihttp://hdl.handle.net/10198/30137
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherElsevierpt_PT
dc.relationCentre for Environmental and Marine Studies
dc.relationCentre for Environmental and Marine Studies
dc.relationCentre for Environmental and Marine Studies
dc.relationHOPE: HousehOld Particulate mattEr: sources, chemical composition and toxicity.
dc.rights.urihttp://creativecommons.org/licenses/by-nc/4.0/pt_PT
dc.subjectDosept_PT
dc.subjectDosimetry modelspt_PT
dc.subjectParticulate matterpt_PT
dc.subjectPM depositionpt_PT
dc.subjectSchoolchildrenpt_PT
dc.titleSeasonal variation in exposure to particulate matter among children attending different levels of education: comparison of two dosimetry modelspt_PT
dc.typejournal article
dspace.entity.typePublication
oaire.awardTitleCentre for Environmental and Marine Studies
oaire.awardTitleCentre for Environmental and Marine Studies
oaire.awardTitleCentre for Environmental and Marine Studies
oaire.awardTitleHOPE: HousehOld Particulate mattEr: sources, chemical composition and toxicity.
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F50017%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F50017%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/LA%2FP%2F0094%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/CEEC IND5ed/2022.00399.CEECIND%2FCP1720%2FCT0012/PT
oaire.citation.endPage12pt_PT
oaire.citation.issue9pt_PT
oaire.citation.startPage1pt_PT
oaire.citation.titleAtmospheric Pollution Researchpt_PT
oaire.citation.volume15pt_PT
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStreamCEEC IND5ed
person.familyNameFeliciano
person.givenNameManuel
person.identifier.ciencia-id2D11-7230-702B
person.identifier.orcid0000-0002-3147-4511
person.identifier.scopus-author-id6603358480
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
rcaap.rightsopenAccesspt_PT
rcaap.typearticlept_PT
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