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From nano- to macro-scale: hybrid magnetic carbon nanocomposites as a tool for catalytic wet peroxide oxidation

dc.contributor.authorRibeiro, Rui
dc.contributor.authorSilva, Adrián
dc.contributor.authorFaria, Joaquim
dc.contributor.authorGomes, Helder
dc.date.accessioned2020-01-15T09:57:36Z
dc.date.available2020-01-15T09:57:36Z
dc.date.issued2018
dc.description.abstractThere is a need for technological innovation in the water sector worldwide, as a result of the growing demand for water supplies – meeting increasingly restricted quality criteria, while coping with the increasing scarcity of clean water sources1. Under this context, the use of treated wastewater as an alternative water source has emerged as a topic of high priority2. However, meeting current quality requirements for wastewater reuse is a great challenge, in which nanotechnology holds a great potential1. Catalytic wet peroxide oxidation (CWPO) is a promising water/wastewater treatment technology; it enables the formation of highly oxidizing hydroxyl radicals (HO•) under atmospheric pressure and low to moderate temperatures, when a suitable catalyst is employed for the decomposition of hydrogen peroxide (H2O2)3. However, further improvement of catalyst design is still required in order to allow the scale-up of the CWPO technology towards real-scale applications. Bearing this in mind, our work has been focused on the development of highly active and stable hybrid magnetic carbon nanocomposites for CWPO. A detailed catalyst design at the nanoscale, based on the understanding of the surface reactions and interactions involved in the CWPO process, has recently allowed us to move forward towards the treatment of a real industrial wastewater with high pollutant load – collected from a mechanical biological treatment (MBT) plant for municipal solid waste processing. This communication reports the findings obtained in the last four years by our research group in this quest. A particular emphasis is given to the synergistic effects arising from the combination of iron-based catalysts with the easily tuned properties of carbon-based materials.pt_PT
dc.description.sponsorshipThis work was supported by: Project POCI-01-0145-FEDER-006984 – Associate Laboratory LSRE-LCM funded by FEDER through COMPETE2020 – Programa Operacional Competitividade e Internacionalização (POCI) – and by national funds through FCT – Fundação para a Ciência e a Tecnologia. R.S. Ribeiro acknowledges the FCT individual Ph.D. grant SFRH/BD/94177/2013, with financing from FCT and the European Social Fund (through POPH and QREN).pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.citationRibeiro, Rui; Silva, Adrián; Faria, Joaquim; Gomes, Helder (2018). From nano- to macro-scale: hybrid magnetic carbon nanocomposites as a tool for catalytic wet peroxide oxidation. In Carbon 2018: book of abstracts. Madridpt_PT
dc.identifier.urihttp://hdl.handle.net/10198/20373
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.rights.urihttp://creativecommons.org/licenses/by-nc/4.0/pt_PT
dc.titleFrom nano- to macro-scale: hybrid magnetic carbon nanocomposites as a tool for catalytic wet peroxide oxidationpt_PT
dc.typeconference object
dspace.entity.typePublication
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/SFRH/SFRH%2FBD%2F94177%2F2013/PT
oaire.citation.conferencePlaceMadrid, Espanhapt_PT
oaire.citation.titleCarbon 2018pt_PT
oaire.fundingStreamSFRH
person.familyNameGomes
person.givenNameHelder
person.identifier.ciencia-id6218-1E19-13EE
person.identifier.orcid0000-0001-6898-2408
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.nameFundação para a Ciência e a Tecnologia
rcaap.rightsopenAccesspt_PT
rcaap.typeconferenceObjectpt_PT
relation.isAuthorOfPublication0eb96337-224a-4339-9918-334436fbbb99
relation.isAuthorOfPublication.latestForDiscovery0eb96337-224a-4339-9918-334436fbbb99
relation.isProjectOfPublication87df9a8b-083c-4efd-832f-32e56b5b6c1e
relation.isProjectOfPublication.latestForDiscovery87df9a8b-083c-4efd-832f-32e56b5b6c1e

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