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Purification of green hydrogen from natural gas grids using zeolite 13X

2023Comunicação em conferência Acesso aberto
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dc.contributor.authorZafanelli, Lucas F.A.S.
dc.contributor.authorHenrique, Adriano
dc.contributor.authorAly, Ezzeldin
dc.contributor.authorRodrigues, Alírio
dc.contributor.authorSilva, José A.C.
dc.date.accessioned2025-01-17T16:35:37Z
dc.date.available2025-01-17T16:35:37Z
dc.date.issued2023
dc.description.abstractGreen hydrogen (GH) is a hot topic in the shift to clean energy, holding a promise to meet global energy demand while contributing to climate action goals. Its transportation can be done into Natural Gas (NG) grids, being necessary a separation technology to provide pure GH and NG to the end user. Accordingly, in this work, a series of breakthrough experiments evaluated the performance of binder-free zeolite 13X as a potential adsorbent to purify GH blended into NG grids. Single and multicomponent experiments were performed at 195, 231, and 273 K and pressure up to 1800 kPa. Noteworthy, the material enables a thermodynamic-based separation of these components due to its strong interaction with CH4, resulting in selectivity values up to 17 at 195 K. The dual-site and standard Langmuir isotherm models fitted the adsorption equilibrium data, being the simulated multicomponent breakthrough curves suitably predicted by a homemade dynamic mathematical model.pt_PT
dc.description.sponsorshipThe authors are grateful to the Foundation for Science and Technology (FCT, Portugal) under project PTDC 2020 * 3599-PPCDTI * Engenharia dos Processos Químicos * project PTDC/EQU-EPQ/0467/2020. Also, through national funds FCT/MCTES (PIDDAC) to CIMO (UIDB/00690/2020 and UIDB/00690/2020), SusTEC (LA/P/0007/ 2021), ALiCE (LA/P/0045/2020), and LSRE-LCM (UIDB/50020/2020 and UIDP/50020/2020). Additionally, we thank national funding by FCT through the individual PhD research grant SFRH/BD/7925/2020 of Lucas F. A. S. Zafanelli. Moreover, the authors are grateful to Kristin Gleichmann and Chemiewerk Bad Koestritz GmbH for kindly providing the binder-free beads of zeolite 13X studied in this work.pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.citationZafanelli, Lucas F.A.S.; Henrique, Adriano; Aly, Ezzeldin; Rodrigues, Alírio; Silva, José A.C. (2023). Purification of green hydrogen from natural gas grids using zeolite 13X. In 6th International Conference Wastes: Solutions, Treatments and Opportunities. Abingdon: CRC Press. p. 63-68. ISBN 978-1-032-38442-9pt_PT
dc.identifier.doi10.1201/9781003345084-11pt_PT
dc.identifier.isbn9781003345084
dc.identifier.urihttp://hdl.handle.net/10198/31024
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherCRC Presspt_PT
dc.relationSFRH/BD/7925/2020pt_PT
dc.relationGreen Hydrogen Separation from Natural Gas Grids by Adsorption Processes with MOFs
dc.relationMountain Research Center
dc.relationALICE - Associate Laboratory in Chemical Engineering
dc.relationLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
dc.relationLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/pt_PT
dc.subjectHydrogen purificationpt_PT
dc.subjectProcess simulationpt_PT
dc.subjectNatural gas grispt_PT
dc.subjectHydrogen recoverypt_PT
dc.subjectGreen hydrogenpt_PT
dc.titlePurification of green hydrogen from natural gas grids using zeolite 13Xpt_PT
dc.typeconference paper
dspace.entity.typePublication
oaire.awardTitleGreen Hydrogen Separation from Natural Gas Grids by Adsorption Processes with MOFs
oaire.awardTitleMountain Research Center
oaire.awardTitleALICE - Associate Laboratory in Chemical Engineering
oaire.awardTitleLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
oaire.awardTitleLaboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/Concurso para Financiamento de Projetos de Investigação Científica e Desenvolvimento Tecnológico em Todos os Domínios Científicos - 2020/PTDC%2FEQU-EPQ%2F0467%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F00690%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/LA%2FP%2F0045%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F50020%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F50020%2F2020/PT
oaire.citation.conferencePlaceCoimbrapt_PT
oaire.citation.title6th International Conference Wastes: Solutions, Treatments and Opportunitiespt_PT
oaire.fundingStreamConcurso para Financiamento de Projetos de Investigação Científica e Desenvolvimento Tecnológico em Todos os Domínios Científicos - 2020
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
person.familyNameZafanelli
person.familyNameHenrique
person.familyNameAly
person.familyNameSilva
person.givenNameLucas F.A.S.
person.givenNameAdriano
person.givenNameEzzeldin
person.givenNameJosé A.C.
person.identifier.ciencia-id3D11-114D-1019
person.identifier.ciencia-idDB18-4E7D-6696
person.identifier.ciencia-idC11B-F5CF-7C78
person.identifier.orcid0000-0001-5187-2042
person.identifier.orcid0000-0002-5227-9790
person.identifier.orcid0000-0003-4840-2597
person.identifier.orcid0000-0003-1778-3833
person.identifier.scopus-author-id7403023684
project.funder.identifierhttp://doi.org/10.13039/501100001871
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project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
rcaap.rightsopenAccesspt_PT
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